(Q38867180)

7 September 2017

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title

Oxidation Reactions with Bioinspired Mononuclear Non-Heme Metal-Oxo Complexes (English)

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7 September 2017

Xenia Engelmann

1

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7 September 2017

Inés Monte-Pérez

series ordinal

2

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7 September 2017

Kallol Ray

series ordinal

3

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7 September 2017

language of work or name

English

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publication date

16 June 2016

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Angewandte Chemie International Edition

7 September 2017

published in

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volume

55

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7 September 2017

issue

27

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7 September 2017

page(s)

7632-7649

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Photoelectrochemical cells

7 September 2017

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Beyond oil and gas: the methanol economy

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Platinum catalysts for the high-yield oxidation of methane to a methanol derivative

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Cellulose degradation by polysaccharide monooxygenases.

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High-valent metal-oxo intermediates in energy demanding processes: from dioxygen reduction to water splitting

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Photosynthetic water oxidation: insights from manganese model chemistry

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Structure of the key species in the enzymatic oxidation of methane to methanol

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Dioxygen activation in soluble methane monooxygenase

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[CuO](+) and [CuOH](2+) complexes: intermediates in oxidation catalysis?

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Evidence for oxygen binding at the active site of particulate methane monooxygenase.

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Structural and mechanistic insights into methane oxidation by particulate methane monooxygenase

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Low temperature syntheses and reactivity of Cu2O2 active-site models

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Developing mononuclear copper-active-oxygen complexes relevant to reactive intermediates of biological oxidation reactions

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Mononuclear Cu-O2 complexes: geometries, spectroscopic properties, electronic structures, and reactivity

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Bis(mu-oxo)dimetal "diamond" cores in copper and iron complexes relevant to biocatalysis

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Copper dioxygen (bio)inorganic chemistry

21 January 2018

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Quantum mechanical calculations suggest that lytic polysaccharide monooxygenases use a copper-oxyl, oxygen-rebound mechanism

21 January 2018

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Catalytic mechanism of dopamine beta-monooxygenase mediated by Cu(III)-oxo.

21 January 2018

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Dioxygen activation by copper, heme and non-heme iron enzymes: comparison of electronic structures and reactivities

21 January 2018

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Elaboration of copper-oxygen mediated C-H activation chemistry in consideration of future fuel and feedstock generation

21 January 2018

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Tuning reactivity and mechanism in oxidation reactions by mononuclear nonheme iron(IV)-oxo complexes

21 January 2018

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Role of metal-oxo complexes in the cleavage of C-H bonds

21 January 2018

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Primary amine stabilization of a dicopper(III) bis(μ-oxo) species: modeling the ligation in pMMO.

21 January 2018

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Formation of hybrid guanidine-stabilized bis(μ-oxo)dicopper cores in solution: Electronic and steric perturbations.

21 January 2018

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Phenolate hydroxylation in a bis(mu-oxo)dicopper(III) complex: lessons from the guanidine/amine series

21 January 2018

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Hydrocarbon hydroxylation by cytochrome P450 enzymes

21 January 2018

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Cytochrome P450 Compound I: Capture, Characterization, and C-H Bond Activation Kinetics

21 January 2018

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https://api.crossref.org/works/10.1002%2FANIE.201600507

Theoretical perspective on the structure and mechanism of cytochrome P450 enzymes.

21 January 2018

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https://api.crossref.org/works/10.1002%2FANIE.201600507

Hydrogen Atom Abstraction by Permanganate: Oxidations of Arylalkanes in Organic Solvents

21 January 2018

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https://api.crossref.org/works/10.1002%2FANIE.201600507

Do Spin State and Spin Density Affect Hydrogen Atom Transfer Reactivity?

21 January 2018

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https://api.crossref.org/works/10.1002%2FANIE.201600507

The first direct characterization of a high-valent iron intermediate in the reaction of an alpha-ketoglutarate-dependent dioxygenase: a high-spin FeIV complex in taurine/alpha-ketoglutarate dioxygenase (TauD) from Escherichia coli

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Direct spectroscopic detection of a C-H-cleaving high-spin Fe(IV) complex in a prolyl-4-hydroxylase

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Direct spectroscopic evidence for a high-spin Fe(IV) intermediate in tyrosine hydroxylase

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Substrate-triggered formation and remarkable stability of the C-H bond-cleaving chloroferryl intermediate in the aliphatic halogenase, SyrB2

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Non-heme Fe(IV)-oxo intermediates

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Direct detection of oxygen intermediates in the non-heme Fe enzyme taurine/alpha-ketoglutarate dioxygenase.

21 January 2018

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https://api.crossref.org/works/10.1002%2FANIE.201600507

High-valent iron(IV)-oxo complexes of heme and non-heme ligands in oxygenation reactions

21 January 2018

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https://api.crossref.org/works/10.1002%2FANIE.201600507

The road to non-heme oxoferryls and beyond

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

A synthetic high-spin oxoiron(IV) complex: generation, spectroscopic characterization, and reactivity

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

A more reactive trigonal-bipyramidal high-spin oxoiron(IV) complex with a cis-labile site

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Modeling TauD-J: a high-spin nonheme oxoiron(IV) complex with high reactivity toward C-H bonds

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Formation, structure, and EPR detection of a high spin Fe(IV)-oxo species derived from either an Fe(III)-oxo or Fe(III)-OH complex.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Spectroscopic and quantum chemical studies on low-spin FeIV=O complexes: Fe-O bonding and its contributions to reactivity

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Nuclear resonance vibrational spectroscopy on the Fe(IV)=O S=2 non-heme site in TMG3tren: experimentally calibrated insights into reactivity

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Excited state potential energy surfaces and their interactions in Fe(IV)=O active sites

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

A two-state reactivity rationale for counterintuitive axial ligand effects on the C-H activation reactivity of nonheme FeIV=O oxidants

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

The fundamental role of exchange-enhanced reactivity in C-H activation by S=2 oxo iron(IV) complexes

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

[Fe(IV)═O(TBC)(CH3CN)]2+: comparative reactivity of iron(IV)-oxo species with constrained equatorial cyclam ligation.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

C-H Bond Cleavage by Bioinspired Nonheme Oxoiron(IV) Complexes, Including Hydroxylation of n-Butane.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Iron-catalyzed halogenation of alkanes: modeling of nonheme halogenases by experiment and DFT calculations

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Substrate-triggered activation of a synthetic [Fe2(μ-O)2] diamond core for C-H bond cleavage

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

An FeIV=O complex of a tetradentate tripodal nonheme ligand

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Crystallographic and Spectroscopic Characterization of a Nonheme Fe(IV)&cjs0811;O Complex

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Axial ligand substituted nonheme FeIV=O complexes: observation of near-UV LMCT bands and Fe=O Raman vibrations.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Axial ligand effects on the geometric and electronic structures of nonheme oxoiron(IV) complexes

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Axial ligand tuning of a nonheme iron(IV)-oxo unit for hydrogen atom abstraction

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

An Ultra-Stable Oxoiron(IV) Complex and Its Blue Conjugate Base.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Contrasting cis and trans effects on the reactivity of nonheme oxoiron(IV) complexes.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Nonheme Oxoiron(IV) Complexes of Pentadentate N5 Ligands: Spectroscopy, Electrochemistry, and Oxidative Reactivity

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Nonheme Fe(IV) Oxo Complexes of Two New Pentadentate Ligands and Their Hydrogen-Atom and Oxygen-Atom Transfer Reactions.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Structures of Nonheme Oxoiron(IV) Complexes from X-ray Crystallography, NMR Spectroscopy, and DFT Calculations

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Evidence that steric factors modulate reactivity of tautomeric iron-oxo species in stereospecific alkane C-H hydroxylation

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Formation of a room temperature stable Fe(V)(O) complex: reactivity toward unactivated C-H bonds

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Activation parameters as mechanistic probes in the TAML iron(V)-oxo oxidations of hydrocarbons

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

A highly reactive p450 model compound I.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Crystal structure of a metal ion-bound oxoiron(IV) complex and implications for biological electron transfer.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Sc3+-triggered oxoiron(IV) formation from O2 and its non-heme iron(II) precursor via a Sc3+-peroxo-Fe3+ intermediate.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

A change in the oxidation state of iron: scandium is not innocent

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Lewis Acid Coupled Electron Transfer of Metal-Oxygen Intermediates.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Unified view of oxidative C-H bond cleavage and sulfoxidation by a nonheme iron(IV)-oxo complex via Lewis acid-promoted electron transfer.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Mechanistic borderline of one-step hydrogen atom transfer versus stepwise Sc(3+)-coupled electron transfer from benzyl alcohol derivatives to a non-heme iron(IV)-oxo complex

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Metal ion effect on the switch of mechanism from direct oxygen transfer to metal ion-coupled electron transfer in the sulfoxidation of thioanisoles by a non-heme iron(IV)-oxo complex.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Proton-promoted oxygen atom transfer vs proton-coupled electron transfer of a non-heme iron(IV)-oxo complex

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Brønsted acid-promoted C-H bond cleavage via electron transfer from toluene derivatives to a protonated nonheme iron(IV)-oxo complex with no kinetic isotope effect

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Efficient Epoxidation of Styrene Derivatives by a Nonheme Iron(IV)-Oxo Complex via Proton-Coupled Electron Transfer with Triflic Acid

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Ferryl protonation in oxoiron(IV) porphyrins and its role in oxygen transfer

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Nonheme FeIVO complexes that can oxidize the C-H bonds of cyclohexane at room temperature.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Chemical and Spectroscopic Evidence for an FeV-Oxo Complex

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

One-electron oxidation of an oxoiron(IV) complex to form an [O═FeV═NR]+ center.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Trapping a Highly Reactive Nonheme Iron Intermediate That Oxygenates Strong C-H Bonds with Stereoretention.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Structure of dipotassium ferrate(VI)

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Does a higher metal oxidation state necessarily imply higher reactivity toward H-atom transfer? A computational study of C-H bond oxidation by high-valent iron-oxo and -nitrido complexes.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

(TAML)FeIV O complex in aqueous solution: synthesis and spectroscopic and computational characterization

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Dichotomous hydrogen atom transfer vs proton-coupled electron transfer during activation of X-H bonds (X = C, N, O) by nonheme iron-oxo complexes of variable basicity

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Lessons from Nature: A Bio-Inspired Approach to Molecular Design

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Nucleophilic attack of hydroxide on a Mn(V) oxo complex: a model of the O-O bond formation in the oxygen evolving complex of photosystem II.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Applications of transition-metal catalysts to textile and wood-pulp bleaching

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

A mononuclear non-heme manganese(IV)-oxo complex binding redox-inactive metal ions.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Enhanced electron-transfer reactivity of nonheme manganese(IV)-oxo complexes by binding scandium ions.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Tuning the Reactivity of Mononuclear Nonheme Manganese(IV)-Oxo Complexes by Triflic Acid

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Preparation and properties of a monomeric high-spin Mn(V)-oxo complex

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

High-spin Mn-oxo complexes and their relevance to the oxygen-evolving complex within photosystem II.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

C-H bond cleavage with reductants: re-investigating the reactivity of monomeric Mn(III/IV)-oxo complexes and the role of oxo ligand basicity

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Proton-Promoted and Anion-Enhanced Epoxidation of Olefins by Hydrogen Peroxide in the Presence of Nonheme Manganese Catalysts.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Preparation and properties of a monomeric Mn(IV)-oxo complex

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

The Catalytic Mechanism of Peptidylglycine α-Hydroxylating Monooxygenase Investigated by Computer Simulation

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Computational exploration of the catalytic mechanism of dopamine beta-monooxygenase: modeling of its mononuclear copper active sites

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Copper(I)-alpha-ketocarboxylate complexes: characterization and O2 reactions that yield copper-oxygen intermediates capable of hydroxylating arenes

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Generating Cu(II)-oxyl/Cu(III)-oxo species from Cu(I)-alpha-ketocarboxylate complexes and O2: in silico studies on ligand effects and C-H-activation reactivity

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

CopperII-mediated aromatic ortho-hydroxylation: a hybrid DFT and AB initio exploration

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Copper-hydroperoxo-mediated N-debenzylation chemistry mimicking aspects of copper monooxygenases

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Quantum chemical assessment of the binding energy of CuO+.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Penetrating the Elusive Mechanism of Copper-Mediated Fluoromethylation in the Presence of Oxygen through the Gas-Phase Reactivity of Well-Defined [LCuO](+) Complexes with Fluoromethanes (CH(4-n)Fn, n = 1-3).

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Lewis acid trapping of an elusive copper-tosylnitrene intermediate using scandium triflate

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Evidence of two-state reactivity in alkane hydroxylation by Lewis-acid bound copper-nitrene complexes

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Rapid C-H bond activation by a monocopper(III)-hydroxide complex

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Hydrogen atom abstraction from hydrocarbons by a copper(III)-hydroxide complex

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Selective Intermolecular Carbon-Hydrogen Bond Activation by Synthetic Metal Complexes in Homogeneous Solution

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Oxidation of ethane to ethanol by N2O in a metal-organic framework with coordinatively unsaturated iron(II) sites

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Chemical Plausibility of Cu(III) with Biological Ligation in pMMO.

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Molecular designs for controlling the local environments around metal ions

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Rationally tuning the reduction potential of a single cupredoxin beyond the natural range

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

An Fe2IVO2 Diamond Core Structure for the Key Intermediate Q of Methane Monooxygenase

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Electronic structure analysis of multistate reactivity in transition metal catalyzed reactions: the case of C–H bond activation by non-heme iron(iv)–oxo cores

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Mechanism of Taurine: α-Ketoglutarate Dioxygenase (TauD) fromEscherichia coli

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Two interconverting Fe(IV) intermediates in aliphatic chlorination by the halogenase CytC3

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Electronic structure and spectroscopy of “superoxidized” iron centers in model systems: theoretical and experimental trends

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Methane-to-Methanol Conversion by First-Row Transition-Metal Oxide Ions: ScO+, TiO+, VO+, CrO+, MnO+, FeO+, CoO+, NiO+, and CuO+

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Diatomic [CuO]+ and Its Role in the Spin-Selective Hydrogen- and Oxygen-Atom Transfers in the Thermal Activation of Methane

21 January 2018

1 reference

https://api.crossref.org/works/10.1002%2FANIE.201600507

Evidence for a Precursor Complex in CH Hydrogen Atom Transfer Reactions Mediated by a Manganese(IV) Oxo Complex

21 January 2018

1 reference

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21 January 2018

Identifiers

DOI

10.1002/ANIE.201600507

1 reference

7 September 2017

1 reference